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- W1969888618 abstract "The structure of silicate glasses and the corresponding liquids at high pressure and their structure−property relations remain difficult questions in modern physical chemistry, geochemistry, and condensed matter physics. Here we report high- resolution solid-state O-17 3QMAS NMR spectra for mixed cation Ca−Na silicate glasses quenched from melts at high pressure up to 8 GPa. The spectra provide the experimental evidence for the varying pressure-dependence in two different types of nonbridging oxygen (NBO) environments (i.e., Na−O−Si and mixed {Ca,Na}−O−Si) in the single glass composition. The percentage of NBO drops significantly with increasing pressure and is a complex function of melt composition, including cation field strength of network modifying cations. A decrease in NBO fraction with pressure is negatively correlated with the element partitioning coefficient between crystals and liquids at high pressure." @default.
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- W1969888618 date "2008-08-20" @default.
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- W1969888618 title "Oxygen-17 Nuclear Magnetic Resonance Study of the Structure of Mixed Cation Calcium−Sodium Silicate Glasses at High Pressure: Implications for Molecular Link to Element Partitioning between Silicate Liquids and Crystals" @default.
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- W1969888618 doi "https://doi.org/10.1021/jp804458e" @default.
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