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• W1969970835 abstract "• Solvation dynamics in nanoscale solvophobic pore placed in bulk subcritical solvent. • Drying–wetting competition accelerates solvation dynamics in pore compared to bulk. • Timescale of long-time solvation component increases linearly with pore-width. We study using computer simulations the solvation dynamics of a solvophilic solute in a solvophobic nano-confinement placed in equilibrium bulk subcritical liquid near liquid–gas phase-coexistence. We find a bi-exponential solvent response inside the confinement as in the bulk. The solvation timescales are significantly shorter under strong confinement compared to the bulk timescale. This is for a low density fluid phase created via competition between drying effect by the solvophobic walls and the surface-mediated wetting by the solvophilic solute. The timescale increases linearly with slit separation to approach the bulk value. We rationalize our observations by simple hydrodynamic arguments." @default.
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• W1969970835 date "2014-01-01" @default.
• W1969970835 modified "2023-09-24" @default.
• W1969970835 title "Solvation in nanoscale solvophobic confinement near liquid–gas phase coexistence" @default.
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• W1969970835 doi "https://doi.org/10.1016/j.cplett.2013.12.043" @default.
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