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- W1970088007 abstract "The vertical distributions of the important highly reactive stratospheric species, ClO and HO 2 , have been inferred from Spacelab 3 (May 1985) Atmospheric Trace Molecule Spectroscopy (ATMOS) measurements of more detectable radical and reservoir species. A simple steady state algebraic expression for ClO, utilizing the observed ClONO 2 /NO 2 abundance ratio, approximates the ClO results of a time‐dependent photochemical model at sunset (30°N). Balloon measurements of ClO and comparisons of time‐dependent photochemical model calculations of ClONO 2 and HCl with the corresponding ATMOS profiles suggest that the actual ClO values are less than the time‐dependent model profiles for ClO at sunset and sunrise (47°S). Errors in the current model simulation of the partitioning among the principal free chlorine species (HCl, ClONO 2 , and ClO) are indicated. However, a comparison of model results with observations of HOCl suggests that the calculated ClO abundance is not a significant overestimate of actual values. A similar methodology is applied to inferring the HO 2 distribution, either algebraically using the ATMOS‐measured HO 2 NO 2 /NO 2 abundance ratio or numerically utilizing the time‐dependent model. The algebraic results agree with the time‐dependent model values to better than a factor of 2 at sunrise. The accuracy of the time‐dependent model calculations of HO 2 is suggested by the agreement between model results and ATMOS observations for HO 2 NO 2 and balloon measurements Of HO 2 . This confirms for the first time the procedure suggested previously by a number of authors of deriving HO x abundances from observed fields of O 3 and H 2 O." @default.
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- W1970088007 date "1991-02-20" @default.
- W1970088007 modified "2023-09-27" @default.
- W1970088007 title "Inferring the abundances of ClO and HO<sub>2</sub>from Spacelab 3 Atmospheric Trace Molecule Spectroscopy observations" @default.
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- W1970088007 doi "https://doi.org/10.1029/90jd02369" @default.
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