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• W1970099372 abstract "Catalytic cracking deposition (CCD) of methyldiethoxysilane (MDES) can be used to tune the zeolitic pores over MFI zeolite membranes for H2/CO2 separation. CCD of MDES over MFI zeolite was investigated to reveal the catalytic cracking behavior of silane. The cracking products were found to be strongly influenced by cracking temperature and acid sites. The increases of temperature and acid sites were beneficial to CCD of MDES in the zeolitic pores, which could effectively reduce the pore size of zeolite. H+ ion exchange on MFI zeolite membranes has been adopted to increase acid sites in the membrane layer. The membranes were further modified by on-stream CCD of MDES to improve H2 selectivity. The achieved H2 selectivity over ion-exchanged membranes was much higher than that for MFI zeolite membranes without ion exchange. Typically, an ion-exchanged membrane after CCD modification possessed an H2/CO2 separation factor of 42.6 and H2 permeance of 2.82 × 10–7 mol/m2·s·Pa at 500 °C." @default.
• W1970099372 created "2016-06-24" @default.
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• W1970099372 date "2013-09-03" @default.
• W1970099372 modified "2023-09-26" @default.
• W1970099372 title "Catalytic Cracking Deposition of Methyldiethoxysilane for Modification of Zeolitic Pores in MFI/α-Al₂O₃ Zeolite Membrane with H⁺ Ion Exchange Pretreatment" @default.
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• W1970099372 doi "https://doi.org/10.1021/ie4012563" @default.
• W1970099372 hasPublicationYear "2013" @default.
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