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• W1970410129 abstract "We report simulations of laser-pulse driven many-electron dynamics by means of a simple, heuristic extension of the time-dependent configuration interaction singles (TD-CIS) approach. The extension allows for the treatment of ionizing states as nonstationary states with a finite, energy-dependent lifetime to account for above-threshold ionization losses in laser-driven many-electron dynamics. The extended TD-CIS method is applied to the following specific examples: (i) state-to-state transitions in the LiCN molecule which correspond to intramolecular charge transfer, (ii) creation of electronic wave packets in LiCN including wave packet analysis by pump-probe spectroscopy, and, finally, (iii) the effect of ionization on the dynamic polarizability of H(2) when calculated nonperturbatively by TD-CIS." @default.
• W1970410129 created "2016-06-24" @default.
• W1970410129 creator A5032510191 @default.
• W1970410129 creator A5061906414 @default.
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• W1970410129 date "2009-09-16" @default.
• W1970410129 modified "2023-10-04" @default.
• W1970410129 title "Laser-induced electron dynamics including photoionization: A heuristic model within time-dependent configuration interaction theory" @default.
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• W1970410129 doi "https://doi.org/10.1063/1.3218847" @default.
• W1970410129 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/19778110" @default.
• W1970410129 hasPublicationYear "2009" @default.
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