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• W1970603403 startingPage "341" @default.
• W1970603403 abstract "We develop an expansion for the resonance Raman line shape of a three-level system $|a〉$, $|b〉$, and $|c〉$ in an arbitrary strong radiation field, being perturbed by dephasing collisions with foreign gas particles. The microscopic information relevant to the line broadening is expresssed in terms of a hierarchy of $n$-time correlation functions of the transition dipole operator ($n=2,4,6,dots{}$). To lowest order ($n=2$) the spectrum is expressed in terms of the three ordinary line-shape functions corresponding to the $mathrm{ab}$, $mathrm{bc}$, and $mathrm{ac}$ transitions. The present theory is not restricted to the impact limit and, depending on the collision time scale, may yield very different results from the well-known impact spectra. Explicit calculations of the predicted spectra are presented for a model system." @default.
• W1970603403 created "2016-06-24" @default.
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• W1970603403 date "1982-07-01" @default.
• W1970603403 modified "2023-09-23" @default.
• W1970603403 title "Nonimpact theory of resonance Raman line shapes in strong radiation fields" @default.
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• W1970603403 doi "https://doi.org/10.1103/physreva.26.341" @default.
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