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• W1970762801 abstract "Gas-phase polymerizations have been executed at different temperatures, pressures, and hydrogen concentrations using Me2Si[Ind]2ZrCl2 / methylaluminoxane / SiO2(Pennsylvania Quarts) as a catalyst. The reaction rate curves have been described by a kinetic model, which takes into account the initially increasing polymerization rate. The monomer concentration in the polymer has been calculated with the Flory–Huggins equation. The kinetic parameters have been determined by fitting the reaction rate curves with the model. At high temperatures, pressures, and hydrogen concentrations a runaway on particle scale may occur leading to reduced polymer yields. The molecular weight and molecular weight distribution of the polymer samples could be described by a “two-site model.” At constant temperature the chain-transfer probability of sites 1 and 2 depends only on the hydrogen concentration divided by the monomer concentration. © 2001 John Wiley & Sons, Inc. J Polym Sci A: Polym Chem 39: 500–513, 2001" @default.
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• W1970762801 date "2001-01-01" @default.
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• W1970762801 title "Gas-phase polymerization of propylene: Reaction kinetics and molecular weight distribution" @default.
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• W1970762801 doi "https://doi.org/10.1002/1099-0518(20010215)39:4<500::aid-pola1019>3.0.co;2-s" @default.
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