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- W1970787817 abstract "In this paper we present experimental observations of reaction rate oscillations during CO oxidation over Pt/γ-Al2O3 at atmospheric pressures. Based on our experimental observations and prior experimental literature on this reaction we propose a mechanistic scheme, which we believe explains in qualitative terms the oscillatory behavior exhibited by this catalytic reaction system. This mechanistic scheme involves a Langmuir-Hinshelwood reaction between adsorbed CO and oxygen and a slow formation and reduction step of an inactive surface oxide species. Our experimental observations and mechanistic ideas, furthermore, support the existence of multiple time scale phenomena for this catalytic reaction system, an idea originally suggested by Chang and Aluko." @default.
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- W1970787817 date "1985-02-01" @default.
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- W1970787817 title "Reaction rate oscillations during CO oxidation over Pt/γ-Al2O3; experimental observations and mechanistic causes" @default.
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- W1970787817 doi "https://doi.org/10.1016/0039-6028(85)90660-0" @default.
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