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- W1970909654 abstract "A many-body diagrammatic technique has been applied to the time correlator reformulation of doubly resonant infrared-visible sum-frequency generation in molecules. Multimode model calculations show the ability of such an experiment to probe the excited state potential well of adsorbed species. In principle, it is possible to discrimate between linear and quadratic vibronic couplings and to recover these parameters from the data. In presence of very large inhomogeneous broadening of the electronic transition however, the sensitivity to quadratic couplings is being lost while the usefulness of this technique in surface specific vibrational spectroscopy is being preserved." @default.
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- W1970909654 date "1996-10-01" @default.
- W1970909654 modified "2023-10-18" @default.
- W1970909654 title "A MANY-BODY APPROACH TO DOUBLY RESONANT SUM-FREQUENCY GENERATION INCLUDING QUADRATIC VIBRATIONAL-MODE COUPLINGS" @default.
- W1970909654 doi "https://doi.org/10.1142/s0218863596000519" @default.
- W1970909654 hasPublicationYear "1996" @default.
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