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- W1971373307 abstract "A coupled spin representation is introduced to describe the classical dynamics of two vibrational modes of a polyatomic molecule coupled by Coriolis interaction to overall molecular rotation. The mechanisms of Coriolis-induced periodic energy exchange between the vibrational modes, resonant vibration–rotation interaction, and chaotic energy transfer are described, and the dependence of the dynamics on rotational angular momentum, vibrational energy, total energy, and parameters in the Hamiltonian is explored using classical trajectory integrations and the surface of section method. The integrable motion occuring in the prolate limit is considered geometrically from the coupled spin representation, which provides clear insight into the dynamics of the system. In addition, this approach allows analytic results describing the effect of Coriolis coupling on vibration–rotation dynamics to be obtained." @default.
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- W1971373307 date "1991-03-01" @default.
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- W1971373307 title "Coriolis interaction in polyatomic molecules: A classical coupled spin representation" @default.
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- W1971373307 doi "https://doi.org/10.1063/1.459731" @default.
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