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• W1971686269 abstract "Although it is commonly known that H-type PBI aggregates give rise to a broad, red-shifted excimer fluorescence with considerably longer fluorescence lifetimes than observed for the monomers, the underlying mechanisms of excimer formation and other relevant exciton dynamics in such π-stacked systems are still far from being understood. In this context, we demonstrate a thorough spectroscopic investigation on the exciton relaxation pathways, including excimer formation, in a perylene-3,4:9,10-bis(dicarboximide) (PBI) dimer aggregate 1 by using time-resolved fluorescence and transient absorption spectroscopy combined with excitation-power and polarization dependence. It was found that the excited dimer formation process followed by structural rearrangement is approximately two times faster than observed within larger PBI aggregates. Excitation-power-dependent transient absorption decay profiles revealed the fully delocalized nature of excitons in the dimer as opposed to larger stacks." @default.
• W1971686269 created "2016-06-24" @default.
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• W1971686269 date "2014-10-08" @default.
• W1971686269 modified "2023-09-30" @default.
• W1971686269 title "Spectroscopic Demonstration of Exciton Dynamics and Excimer Formation in a Sterically Controlled Perylene Bisimide Dimer Aggregate" @default.
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• W1971686269 doi "https://doi.org/10.1021/jz501953a" @default.
• W1971686269 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26278616" @default.
• W1971686269 hasPublicationYear "2014" @default.
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