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- W1971952034 abstract "A one-dimensional, time-dependent model has been developed to study the removal of solublegases from a warm, precipitating stratiform cloud. The model calculates the distributions ofwater vapor and condensed water, in the form of cloud drops and raindrops, as well as the incloudconcentration of a soluble species in the gas and aqueous phases for a specified profile ofpressure and temperature and an assumed updraft velocity. Highly soluble gases are found tobe rapidly dissolved into cloud droplets and then slowly incorporated into raindrops ascloudwater is converted to rainwater. As this rainwater begins to fall out of the cloud, the totalin-cloud abundance of highly soluble species rapidly decreases, causing the rate of removal ofthe species from the cloud to also decrease. The rate of removal of highly soluble speciescontinues to decrease until a balance between loss via rainout and transport of new materialinto the cloud is reached, and an approximate steady state is established. Thus the rainout ratefor highly soluble species is found to be ultimately limited by the rate at which new gaseousmaterial can be transferred from the cloud-free air into the cloud. The model calculationsindicate that turbulence represents an important mechanism by which highly soluble gases aretransported into strati form clouds and thus the calculated rate of removal of highly solublespecies from these types of clouds is dependent on the parameterization chosen to simulatethis process. DOI: 10.1111/j.1600-0889.1986.tb00194.x" @default.
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- W1971952034 date "1986-07-09" @default.
- W1971952034 modified "2023-10-17" @default.
- W1971952034 title "The removal of soluble species by warm stratiform clouds" @default.
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- W1971952034 doi "https://doi.org/10.1111/j.1600-0889.1986.tb00194.x" @default.
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