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- W1972016022 abstract "Abstract In this paper, we report on the comprehensive alcohol-/ion-responsive properties of a smart copolymer poly( N -isopropylacrylamide- co -benzo-18-crown-6-acrylamide) (P(NIPAM- co -BCAm)). The orthogonal design method is adopted for experimental design. The experimental results show that alcohol can trigger the shrinking and Ba 2 + can induce the swelling of the P(NIPAM- co -BCAm) copolymer. According to the phase transition temperature (LCST) change results of the copolymer, the influence of variables on the LCST changes weakens in the following order: alcohol concentration > alcohol species > metal ion species > BCAm concentration > ion concentration. The larger the alcohol concentration and the larger the molecular size of alcohols, the lower the LCST value; on the contrary, the more the BCAm content in the copolymer or the larger the BCAm/ion complex stability constant (lg K ) or the larger the ion concentration is, the higher the LCST value. For a P(NIPAM- co -BCAm) copolymer with a fixed BCAm content, a binary function of ion concentration and lg K of BCAm/ion is developed to precisely predict the LCST values of the copolymer in different metal ion solutions. The results provide valuable information for fabricating artificial biomimetic G-protein-gated inwardly rectifying potassium (GIRK) channels that are activated by alcohol and inhibited by Ba 2 + ." @default.
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- W1972016022 date "2014-09-01" @default.
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- W1972016022 title "Comprehensive Alcohol-/Ion-Responsive Properties of Poly(N-Isopropylacrylamide-co-Benzo-18-Crown-6-Acrylamide) Copolymers" @default.
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- W1972016022 doi "https://doi.org/10.1016/j.cjche.2014.06.021" @default.
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