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• W1972038296 abstract "The recently discovered ring-opening polymerization (ROP) of β-butyrolactone (β-BL) using CrIII(salphen) as catalyst converts racemic β-BL to isotactic enriched poly(hydroxybutyrate) (PHB). These achiral complexes arrange themselves in a dimeric sandwich-like structure entrapping the growing polymer chain and the monomer. The polymerization mechanism discussed based on previous DFT calculations is supported by kinetic studies in here. Furthermore, the influence of different substitution patterns in salphen complexes on polymerization of β-BL was investigated. In addition, effects of different polymerization starters and additives on the broad molecular weight distribution of PHB have been investigated, which show the limitations of this catalysis." @default.
• W1972038296 created "2016-06-24" @default.
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• W1972038296 date "2010-10-22" @default.
• W1972038296 modified "2023-10-17" @default.
• W1972038296 title "Factors Influencing the Ring-Opening Polymerization of Racemic β-Butyrolactone Using Cr^III(salphen)" @default.
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• W1972038296 doi "https://doi.org/10.1021/ma101407r" @default.
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