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- W1972070280 abstract "The fluorescence excitation spectrum of the lowest excited 1B3u(n π*) state of pyrazine cooled in a pulsed supersonic free jet was observed. The fluorescence decay of the isolated molecule was also measured in the free jet. The rotationally cooled pyrazine in the collision free condition exhibits extremely large fluorescence quantum yield and dominant slow fluorescence component for low lying vibronic levels. The ratio of the pre-exponential factors of the dual fluorescence decay was examined in terms of the available theory of singlet-triplet mixed state model. It was found that the number of coupled triplet levels obtained from the observed ratio is inconsistent with the calculated excess energy dependence of vibronic density in the triplet state. Remarkable rotational level dependence of the ratio of the pre-exponential factors was observed for the electronic origin, while such a rotational dependence was not found for the lifetime of the slow fluorescence." @default.
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- W1972070280 date "1982-02-01" @default.
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- W1972070280 title "Dual Fluorescence of Pyrazine Cooled in a Supersonic Free Jet" @default.
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- W1972070280 doi "https://doi.org/10.1246/bcsj.55.374" @default.
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