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- W1972180530 abstract "Abstract Free doubly-charged negative molecules are a challenge for both theory and experiment. Their stability depends on a very delicate balance between interatomic structure, electronic interaction and Coulomb repulsion. Detecting di-anions of mass M with conventional mass spectrometry always bears the risk of erroneously measuring contributions from singly charged negative ions near mass M /2, or from molecular fragments with different energy. Another possible source of errors are mass ambiguities, e.g. M( 12 C 4 )≈M( 16 O 3 ). In this contribution we show how one can overcome the methodical limits of conventional mass spectrometry by using AMS techniques for the analysis of very rare doubly-charged negative molecules. As an example, a new class of di-anions will be presented, (OC n ) 2− , n ⩾5, which were discovered recently by secondary ion mass spectrometry, and were analyzed in detail by AMS." @default.
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- W1972180530 date "2004-08-01" @default.
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- W1972180530 title "Analysis of doubly-charged negative molecules by accelerator mass spectrometry" @default.
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- W1972180530 doi "https://doi.org/10.1016/j.nimb.2004.04.045" @default.
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