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- W1972306649 abstract "An extensive review of the literature on the high temperature reactions (both in melts and in the solid state) of uranium oxides (UO2, U3O8 and UO3) resulting in the formation of insoluble alkali metal (Li to Cs) uranates is presented. Their uranate(VI) and uranate(V) compounds are examined, together with mixed and oxygen-deficient uranates. The reactions of uranium oxides with carbonates, oxides, per- and superoxides, chlorides, sulfates, nitrates and nitrites under both oxidising and non-oxidising conditions are critically examined and systematised, and the established compositions of a range of uranate(VI) and (V) compounds formed are discussed. Alkali metal uranates(VI) are examined in detail and their structural, physical, thermodynamic and spectroscopic properties considered. Chemical properties of alkali metal uranates(VI), including various methods for their reduction, are also reported. Errors in the current theoretical treatment of uranate(VI) spectra are identified and the need to develop routes for the preparation of single crystals is stressed." @default.
- W1972306649 created "2016-06-24" @default.
- W1972306649 creator A5016309862 @default.
- W1972306649 creator A5086003330 @default.
- W1972306649 date "1999-09-01" @default.
- W1972306649 modified "2023-09-27" @default.
- W1972306649 title "A review of the high temperature oxidation of uranium oxides in molten salts and in the solid state to form alkali metal uranates, and their composition and properties" @default.
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