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- W1973095770 abstract "High-pressure X-ray photoelectron spectroscopy, mass spectrometry, and density functional theory calculations have been combined to study methane oxidation over Pd(100). The measurements reveal a high activity when a two-layer PdO(101) oriented film is formed. Although a one-layer PdO(101) film exhibits a similar surface structure, no or very little activity is observed. The calculations show that the presence of an oxygen atom directly below the coordinatively unsaturated Pd atom in the two-layer PdO(101) film is crucial for efficient methane dissociation, demonstrating a ligand effect that may be broadly important in determining the catalytic properties of oxide thin films." @default.
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- W1973095770 date "2014-08-28" @default.
- W1973095770 modified "2023-10-02" @default.
- W1973095770 title "Intrinsic Ligand Effect Governing the Catalytic Activity of Pd Oxide Thin Films" @default.
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- W1973095770 doi "https://doi.org/10.1021/cs5010163" @default.
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