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• W1973164062 abstract "The “spur lifetime” (τs) in the low-linear energy transfer (LET) radiolysis of supercritical water (SCW) at 400 °C has been determined as a function of water density by using a simple model of energy deposition initially in spurs, followed by the random diffusion (Brownian motion) of the species formed until spur expansion is complete. The values of τs are found to decrease from ∼5.0 × 10−6 to 5.0 × 10−8 s over the density range from 0.15 to 0.6 g cm−3. Using Monte-Carlo simulations, our calculated density dependence of the “escape” hydrated electron (eaq−) yield (i.e., at time τs) reproduces fairly well Bartels and co-workers' scavenged eaq− yield data, suggesting that these data may have been measured at times close to τs." @default.
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• W1973164062 date "2012-01-01" @default.
• W1973164062 modified "2023-09-26" @default.
• W1973164062 title "Density dependence of the “escape” yield of hydrated electrons in the low-LET radiolysis of supercritical water at 400 °C" @default.
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• W1973164062 doi "https://doi.org/10.1039/c2cp41399j" @default.
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