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• W1973353865 abstract "Abstract The real part of third-order optical nonlinearity of an azo dye (2-(2-thiazolylazo)-5-diethylaminophenol, TAEP) and those of its copper- and cobalt-substituted compounds are measured by using femtosecond optical heterodyne optical Kerr gate technique at the wavelength of 647 nm. All the values are found to be negative. Those of Cu- and Co-substituted compounds are found to be larger than that of the metal-free dye by two and three orders of magnitude, respectively. A negative γ eff as large as 10 −29 esu is found in Co complex. We use a three-level model to characterize the nonlinear process, and suggest that π-electron delocalization in metal complex leads to an enhancement." @default.
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• W1973353865 date "2000-11-01" @default.
• W1973353865 modified "2023-10-18" @default.
• W1973353865 title "Investigation of third-order nonlinearity of an azo dye and its metal-substituted compounds" @default.
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• W1973353865 doi "https://doi.org/10.1016/s0009-2614(00)01135-0" @default.
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