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• W1973505363 abstract "The kinetics of the Fe3+/Fe2+ reaction on a Pt rotating disc electrode was studied in solutions of 0.5 M H2SO4 and 0.5 M Na2SO4 (pH 2.2). Taking into account formation of sulphate complexes the conclusion was made that the main contribution to the reaction rate is due to FeSO4+ and FeSO4 complexes. Extended Tafel plots obtained by Randles analysis from experimental current-voltage curves were corrected for the 2 potential. The latter was evaluated according to the Gouy-Chapman theory by using the surface charge density values deduced from thermodynamic theory and measurements of other authors. Tafel plots were approximated by parabolas and the reorganization energy was calculated as 33 kJ mol−1 and 51 kJ mol−1 for Fe3+/Fe2+ in H2SO4 and Na2SO4, respectively. The comparison of these values with theoretically predicted ones was made. From the magnitude of the pre-exponential factor of the true rate constant it was concluded that the Fe3+/Fe2+ electron transfer reaction is non-adiabatic in nature." @default.
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• W1973505363 date "1977-04-01" @default.
• W1973505363 modified "2023-10-18" @default.
• W1973505363 title "The effect of the double layer on the rate of the Fe3+/Fe2+ reaction on a platinum electrode and the contemporary electron transfer theory" @default.
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• W1973505363 doi "https://doi.org/10.1016/s0022-0728(77)80469-5" @default.
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