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• W1973603973 abstract "Computational and experimental results at normal atmospheric pressure are reported for methanol-air premixed and diffusion flames, the latter including fuel streams partially premixed to equivalence ratios down to 2, yielding two-stage flames. Measurements of the concentrations of NOx, of CH4, and of the sum of the concentrations of C2H2, C2H4, and C2H6 (collectively termed C2 species) are made for these flames. By employing 184 elementary steps, 52 of which are associated with the nitrogen chemistry, computations are performed for freely propagating premixed flames with equivalence ratios from 0.5 to 1.9 and for counterflowing two-stage flames with equivalence ratios from 2 to infinity at different initial conditions. Most of the elementary rate constants have been validated in previous experimental and computational studies of H2, CO, CH4, and CH3OH flames. Those that have not mainly concern consumption of CH3O and CH2OH, especially notably CH2OH+H→CH3+OH, which is the dominant reaction leading to the formation of both CH4 and C2 species in these experiments and for which the rate parameters are determined herein. Excellent agreements between experiments and predictions are obtained. This completes the determination of elementary rate parameters for methanol-air flames, to the extent possible on the basis of currently available experimental information, and it thereby provides a reaction mechanism for these flames." @default.
• W1973603973 created "2016-06-24" @default.
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• W1973603973 date "1998-01-01" @default.
• W1973603973 modified "2023-10-16" @default.
• W1973603973 title "Formation of NOx, CH4, and C2 species in laminar methanol flames" @default.
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• W1973603973 doi "https://doi.org/10.1016/s0082-0784(98)80438-4" @default.
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