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• W1973612110 endingPage "1171" @default.
• W1973612110 startingPage "1137" @default.
• W1973612110 abstract "The cascade [1,n]-hydrogen transfer/cyclization, recognized one century ago, has received considerable interest in recent decades and great achievements have been made. This cascade process can functionalize C(sp3)H bonds directly into CC, CN, CO bonds under the catalysis by Lewis acids, Brønsted acids or organocatalysts, and even under thermal conditions. This methodology has shown preeminent power to construct 5- or 6-membered heterocyclic as well as all-carbon rings. In this review, various hydrogen donors and hydrogen acceptors are categorized and discussed. Abbreviations: Cbz: benzyloxycarbonyl; Cod: 1,5-cyclooctadiene; CSA: camphorsulfonic acid; DCE: 1,1-dichloroethane; DFT: density function theory; DMF: N,N-dimethylformamide; DNBS: 2,4-dinitrobenzenesulfonic acid; DPP: diphenyl phosphate; ERC: electrocyclic ring closure; Fmoc: 9-fluorenylmethoxycarbonyl; HT: hydrogen transfer; IBX: ortho-iodoxybenzoic acid; m-CPBA: meta-chloroperbenzoic acid; MW: microwave; MS: molecular sieves; Pg: protecting group; p-TSA: para-toluenesulfonic acid; r.t.: room temperature; TCE: 1,1,2-trichloroethane; TFA: trifluoroacetic acid; TMS: trimethylsilyl." @default.
• W1973612110 created "2016-06-24" @default.
• W1973612110 creator A5044296533 @default.
• W1973612110 creator A5086664647 @default.
• W1973612110 date "2014-03-18" @default.
• W1973612110 modified "2023-10-11" @default.
• W1973612110 title "Advancement in Cascade [1,n]-Hydrogen Transfer/Cyclization: A Method for Direct Functionalization of Inactive C(<i>sp</i>³)H Bonds" @default.
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