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- W1973802210 abstract "The bonding and geometry of CN, NCCN, ethylenediamine, and s-triazine have been investigated with HREELS in order to compare the characteristics of CN bonds of different order on Pd(111) and (100). The CN bond is found to lie parallel to the metal surface in all cases examined. A π-bonded configuration for these adsorbates is likely. The comparison of the single, double and triple bond CN stretch frequencies, ≈130, 190, and 235 meV, respectively, for the chemisorbed species, allows intermediates and reaction products of the more complex CN adsorbates to be identified. CN is the only species resulting from NCCN decomposition on Pd. Ethylenediamine and s-triazine were used to obtain spectra from a compound modelling the “hydrogenation of NCCN” and a “surface polymer”, respectively. On the basis of the spectra of these model compounds, we conclude that a reaction of molecular NCCN with coadsorbed H or the formation of a surface polymer or paracyanogen-like compound from CN does not take place on Pd(111) or (100)." @default.
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- W1973802210 date "1987-08-01" @default.
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- W1973802210 title "A comparison of single-, double-, triple-bonded and aromatic CN compounds on Pd(111) and (100) I. Hreels of NCCN, ethylenediamine and s-triazine" @default.
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- W1973802210 doi "https://doi.org/10.1016/s0039-6028(87)80396-5" @default.
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