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- W1973852114 abstract "We report studies on the controlled step-by-step oxidative functionalization of monolayer graphene by chemically reactive water-vapor plasma dry etching. The use of a porous mask on top of the graphene sheets as a filter is essential to reduce the density of free radicals and weaken the sputtering effect. Micro-Raman spectroscopy, X-ray photoelectron spectroscopy and atomic force microscopy showed that the oxidation occurred in a mild and controllable way, and that a wide variety of oxygen-containing functional groups can be evenly and incrementally incorporated onto the carbon lattice. By monitoring the electrical property changes in the graphene at different levels of oxidation, we observed a transformation of the electrical conduction process from continuum percolation to variable range hopping and/or electric-field-driven tunneling, due to the progressive increase of sp3-based basal plane distortion that disrupts the transport of carriers delocalized in the sp2 carbon network." @default.
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- W1973852114 date "2012-07-01" @default.
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- W1973852114 title "Controlled oxidative functionalization of monolayer graphene by water-vapor plasma etching" @default.
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- W1973852114 doi "https://doi.org/10.1016/j.carbon.2012.02.090" @default.
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