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- W1973992298 abstract "A generalization of the optimized random phase approximation in the thermodynamic perturbation theory of liquids is proposed. By introducing a new method, we can derive an approximate analytical expression for the free energy of simple liquids. This is achieved by invoking a direct correlation function more general than the mean spherical approximation. By correcting the unphysical behavior of the corresponding radial distribution function in the hard core region, we attain a new perturbation expansion as a natural generalization of the optimized random phase approximation. In order to assess its accuracy and reliability, the theory is employed to find the structure and thermodynamics of hard-core Yukawa fluids. The new resulted optimized second order random phase approximation (OSORPA) is shown to be a little more accurate than the optimized random phase approximation in finding the thermodynamic properties, but it performs much better in predicting the static structure factor of hard-core Yukawa potentials." @default.
- W1973992298 created "2016-06-24" @default.
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- W1973992298 date "2015-01-01" @default.
- W1973992298 modified "2023-09-26" @default.
- W1973992298 title "A generalization of random phase approximation as a new theory in the thermodynamic perturbation theory of simple fluids" @default.
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- W1973992298 doi "https://doi.org/10.1016/j.fluid.2014.11.030" @default.
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