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- W1974307925 abstract "The use of tough hydrogels as biomaterials is limited as a consequence of time-consuming fabrication techniques, toxic starting materials, and large strain hysteresis under deformation. Herein, we report the simultaneous application of nucleophilic thiol-yne and inverse electron-demand Diels–Alder additions to independently create two interpenetrating networks in a simple one-step procedure. The resultant hydrogels display compressive stresses of 14–15 MPa at 98% compression without fracture or hysteresis upon repeated load. The hydrogel networks can be spatially and temporally postfunctionalized via radical thiylation and/or inverse electron-demand Diels–Alder addition to residual functional groups within the network. Furthermore, gelation occurs rapidly under physiological conditions, enabling encapsulation of human cells." @default.
- W1974307925 created "2016-06-24" @default.
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- W1974307925 date "2015-01-26" @default.
- W1974307925 modified "2023-10-10" @default.
- W1974307925 title "Simultaneous Orthogonal Dual-Click Approach to Tough, <i>in-Situ</i>-Forming Hydrogels for Cell Encapsulation" @default.
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- W1974307925 doi "https://doi.org/10.1021/ja511681s" @default.
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