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- W1974460704 abstract "We report experiments studying the mechanical evolution of layers of the protein lysozyme adsorbing at the air-water interface using passive and active microrheology techniques to investigate the linear and nonlinear rheological response, respectively. Following formation of a new interface, the linear shear rheology, which we interrogate through the Brownian motion of spherical colloids at the interface, becomes viscoelastic with a complex modulus that has approximately power-law frequency dependence. The power-law exponent characterizing this frequency dependence decreases steadily with increasing layer age. Meanwhile, the nonlinear microrheology, probed via the rotational motion of magnetic nanowires at the interface, reveals a layer response characteristic of a shear-thinning power-law fluid with a flow index that decreases with age. We discuss two possible frameworks for understanding this mechanical evolution: gelation and the formation of a soft glass phase." @default.
- W1974460704 created "2016-06-24" @default.
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- W1974460704 date "2014-01-01" @default.
- W1974460704 modified "2023-09-26" @default.
- W1974460704 title "Linear and nonlinear microrheology of lysozyme layers forming at the air–water interface" @default.
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- W1974460704 doi "https://doi.org/10.1039/c4sm00484a" @default.
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