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- W1974464792 abstract "Abstract Cavity enhanced absorption spectroscopy (CEAS) combined with phase-sensitive detection is employed to study the effects of static magnetic fields on radical recombination reactions. The chemical system comprises the photochemically generated thionine semiquinone radical and a 1,4-diazabicyclo[2.2.2]octane (DABCO) cationic radical in a micellar solution of sodium dodecyl sulphate. Data obtained using the modulated CEAS technique, describing the magnetic field effect (MFE) on reaction yields, are shown to be superior to those obtained using conventional transient absorption (TA) flash photolysis methods typically employed for these measurements. The high sensitivity afforded by modulated CEAS detection is discussed in terms of the new possibilities it offers such as the measurement of magnetic field effects in real biological systems which have hitherto been largely beyond the detection capabilities of existing techniques. Keywords: cavity ring-downcavity enhanced absorptionspin chemistryradical pair mechanismmagnetic field effects Acknowledgements We are grateful for the financial support this work has received from the Engineering and Physical Sciences Research Council (EPSRC), the Royal Society and the EMF Biological Research Trust. SRM is further grateful to the EPSRC for his Advanced Research Fellowship. We are indebted to Professor Ulrich Steiner for helpful discussions." @default.
- W1974464792 created "2016-06-24" @default.
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- W1974464792 date "2010-04-10" @default.
- W1974464792 modified "2023-10-12" @default.
- W1974464792 title "Cavity enhanced detection methods for probing the dynamics of spin correlated radical pairs in solution" @default.
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- W1974464792 doi "https://doi.org/10.1080/00268971003614368" @default.
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