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- W1974481124 abstract "Marked discontinuities are observed in the slope of the variation with gold concentration of the 57Fe isomer shift, linewidth and hyperfine field in the Mossbauer spectra of palladium gold (iron 2 at.%) alloys at around 50 at.% gold. These are associated with a decrease in the effectiveness of charge screening at the iron sites when the palladium d band is filled. The change from ferromagnetic behaviour in palladium iron alloys to random antiferromagnetic behaviour in gold iron alloys is shown to occur when the d band is filled. The observed Curie temperatures of palladium rich alloys are shown to be determined by the matrix susceptibility. A small change in the slope of the 197Au isomer shift variation in palladium gold alloys is observed at about 50 at.% gold which was not seen in the earlier experiment of Roberts et al. There is no anomalous behaviour in the linewidth variation, implying little change in the screening of the gold atoms when the d band is filled. Preliminary measurements on palladium copper (iron 1 at.%) alloys indicate a marked discontinuity in the 57Fe isomer shift variation at 50 at.% copper" @default.
- W1974481124 created "2016-06-24" @default.
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- W1974481124 date "1970-05-01" @default.
- W1974481124 modified "2023-09-24" @default.
- W1974481124 title "A study of band filling in palladium based alloys using the Mossbauer effect in57Fe and197Au" @default.
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- W1974481124 doi "https://doi.org/10.1088/0022-3719/3/1s/309" @default.
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