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- W1974508040 abstract "Based on the theoretical analysis of time-resolved pump-probe spectroscopies we investigate dynamics of the C-O stretching mode of a CO adsorbate on the metal surface incorporating the electron-hole continuum. Asymmetric Fano resonances in the nonlinear spectra are found to evolve in the time domain with a time scale ${ensuremath{tau}}_{mathit{text{Fano}}}$ $[mathcal{O}(0.1)phantom{rule{0.3em}{0ex}}mathrm{ps}ensuremath{sim}mathcal{O}(1)phantom{rule{0.3em}{0ex}}mathrm{ps}]$. ${ensuremath{tau}}_{mathit{text{Fano}}}$ is governed by inherent natures of the electron-hole pair, rather than specific pair creation mechanisms, which means that ${ensuremath{tau}}_{mathit{text{Fano}}}$ is a fundamental time scale in surface dynamics." @default.
- W1974508040 created "2016-06-24" @default.
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- W1974508040 date "2005-11-22" @default.
- W1974508040 modified "2023-09-23" @default.
- W1974508040 title "Nonlinear time-resolved study of dynamics of a CO adsorbate on a metal: Time-evolving Fano resonance with electron-hole continuum" @default.
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- W1974508040 doi "https://doi.org/10.1103/physrevb.72.195111" @default.
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