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• W1974961036 startingPage "4935" @default.
• W1974961036 abstract "The pressure dependence of the ionic conductivity of KCl, NaCl, KBr, and NaBr has been measured to 6 kbar in the intrinsic and extrinsic temperature regions. In the intrinsic region the conductivity deviates markedly from a simple exponential decrease with pressure. A detailed analysis, including contributions from anions and extrinsic cation vacancies, shows that pressure can suppress the intrinsic vacancies sufficiently to cause such a deviation. The analysis also shows that the uncertainties in the estimated activation volumes are greater than those determined in previous work. For KCl, NaCl, KBr, and NaBr crystals, respectively, the estimated activation volumes for motion of cation vacancies are 8 ifmmodepmelsetextpmfi{} 1, 7 ifmmodepmelsetextpmfi{} 1, 11 ifmmodepmelsetextpmfi{} 1, and 8 ifmmodepmelsetextpmfi{} 1 ${mathrm{cm}}^{3}$/mole, and the activation volumes for formation of Schottky defects are 61 ifmmodepmelsetextpmfi{} 9, 55 ifmmodepmelsetextpmfi{} 9, 54 ifmmodepmelsetextpmfi{} 9, and 44 ifmmodepmelsetextpmfi{} 9 ${mathrm{cm}}^{3}$/mole. The values for activation volumes of motion agree with predictions of the strain-energy model of Keyes. Schottky-defect-formation volumes are substantially larger than the molar volumes in KCl and NaCl, but in KBr and NaBr they are approximately equal." @default.
• W1974961036 created "2016-06-24" @default.
• W1974961036 creator A5040153279 @default.
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• W1974961036 date "1972-06-15" @default.
• W1974961036 modified "2023-10-16" @default.
• W1974961036 title "Pressure Dependence of Ionic Conductivity in KCl, NaCl, KBr, and NaBr" @default.
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• W1974961036 doi "https://doi.org/10.1103/physrevb.5.4935" @default.
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