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• W1975431132 abstract "[1] To date, gas photochemistry has not been simulated beyond a few hundred reactions in a three-dimensional (3-D) atmospheric model. Here, we treat 4675 gases and 13,626 tropospheric and stratospheric reactions in the 3-D GATOR-GCMOM climate-pollution model and compare results with data and with results from a condensed 152-gas/297-reaction mechanism when the model was nested at increasing resolution from the globe to California to Los Angeles. Gases included C1-C12 organic degradation products and H-, O-, N-, Cl−, Br-, Fl-, and S-containing inorganics. Organic reactions were from the Master Chemical Mechanism. Photolysis coefficients for 2644 photoprocesses and heating rates for 1909 photolyzing gases were solved with an online radiative code in each grid cell using quantum yield/cross section data over 86 UV/visible wavelengths. Spatial/temporal emissions of > 110 gases were derived from the 2005 U.S. National Emission Inventory. The condensed mechanism was a modified Carbon-Bond IV (MCBIV). Three-day simulation results indicate that the more-explicit mechanism reduced the O3 gross error against data versus the MCBIV error against data by only ∼2 percentage points (from 28.3% to 26.5%) and NO2 and HCHO by ∼6 percentage points in Los Angeles. While more-explicit photochemistry improved results, the condensed mechanism was not the main source of ozone error. The more explicit mechanism, which treated absorptive heating by more photolyzing gases, also resulted in a different magnitude of feedbacks to meteorological variables and back to gases themselves than did the less-explicit mechanism. The computer time for all processes in GATOR-GCMOM with the more explicit mechanism (solved with SMVGEAR II in all domains) was only ∼3.7 times that with the MCBIV despite the factors of 31 and 46 increases in numbers of species and reactions, respectively." @default.
• W1975431132 created "2016-06-24" @default.
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• W1975431132 date "2010-07-27" @default.
• W1975431132 modified "2023-09-24" @default.
• W1975431132 title "Global-through-urban nested three-dimensional simulation of air pollution with a 13,600-reaction photochemical mechanism" @default.
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• W1975431132 doi "https://doi.org/10.1029/2009jd013289" @default.
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