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- W1976991657 abstract "It is shown that proton-acceptor additions are effective inhibitors of the nucleation process of low-temperature decomposition of ammonium perchlorate (AP). In contrast to this, addition of ClO3− ion is a catalyst for the decomposition of AP: It increases the rate of nucleation Vn and the maximum concentration of nuclei Nmax and decreases the induction period of nucleation τ. It is shown that impurity of ClO3− ion is present in the purest commercial samples of AP. It is thought that the initiator of nucleation is HClO3, i.e., Vn = K[H+] × [ClO3−]. The dependence that is demonstrated agrees very well with experimental data on the influence of addition of proton donors and acceptors and of additions of ClO3− ions on Vn. On the basis of this mechanism, means of regulating the temperature of initiation of AP decomposition are suggested. An explanation of the photosensitivity of AP exposed to the uv band is proposed." @default.
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- W1976991657 date "1976-02-01" @default.
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- W1976991657 title "Nucleation mechanism during low-temperature decomposition of ammonium perchlorate" @default.
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- W1976991657 doi "https://doi.org/10.1016/0022-4596(76)90222-x" @default.
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