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• W1977153896 startingPage "2878" @default.
• W1977153896 abstract "This communication describes oxidatively induced Ar-CF(3) bond-forming reductive elimination from new Pd(II) complexes of general structure (L approximately L)Pd(II)(Ar)(CF(3)). The electrophilic fluorinating reagent N-fluoro-2,4,6-trimethylpyridinium triflate promotes these reactions in good to excellent yields. The palladium(IV) intermediate ((t)Bu-bpy)Pd(IV)(CF(3))(F)(OTf)(C(6)H(4)F) has been isolated, characterized, and demonstrated to undergo high yielding Ar-CF(3) coupling upon thermolysis. This work provides an attractive conceptual framework for the development of Pd(II/IV)-catalyzed arene trifluoromethylation reactions." @default.
• W1977153896 created "2016-06-24" @default.
• W1977153896 creator A5028785945 @default.
• W1977153896 creator A5039633479 @default.
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• W1977153896 date "2010-02-15" @default.
• W1977153896 modified "2023-10-01" @default.
• W1977153896 title "Aryl−CF₃ Bond-Forming Reductive Elimination from Palladium(IV)" @default.
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• W1977153896 doi "https://doi.org/10.1021/ja100955x" @default.
• W1977153896 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/2832076" @default.
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