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- W1977156696 abstract "We construct and solve a model of laser photon absorption in polyatomic molecules which is related to the onset of effective intramolecular mode coupling (quasicontinuum). We find coherent absorption of the laser photons despite the many-level nature of the system, however, all of the features of intramolecular vibrational relaxation are also evident if the populations of the pure pumped mode states are monitored as a function of time. The model is also found to be quite stable with respect to an asymmetry in the intramolecular mode coupling constant." @default.
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- W1977156696 date "1983-01-15" @default.
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- W1977156696 title "Coherent pumping in a weakly coupled quasicontinuum model" @default.
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- W1977156696 doi "https://doi.org/10.1063/1.444777" @default.
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