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• W1977176989 abstract "We study the spectral densities for alkali-metal-doped C 60 , A x C 60 ( A =K, Rb, etc), at zero temperature to elucidate the origin of anomalous behaviors in photoemission spectra, based on the dynamical mean-field theory by using the exact diagonalization method. The results for A 2 C 60 and A 4 C 60 agree qualitatively with the results of Hartree–Fock calculations; these materials are insulating due to the cooperation between the electron–electron and electron–phonon interactions. On the contrary, in A 3 C 60 , the competition between the electron–electron and electron–phonon interactions results in the charge fluctuation and consequently the material remains metallic. We find satellites at about 1.6 eV below and above the Fermi level and the enhancement of the spectral intensity at the Fermi level in the spectral density for A 3 C 60 . These originate from the charge fluctuation. Furthermore, it is found that continuous features ranging from -1 eV to +1 eV are derived from the multiplet splitting of C 60 2- and C 60 4- molecules. Our results for A 3 C 60 successfully explain the anomalous behaviors in the photoemission spectra of A 3 C 60 . Moreover, we study the photoemission spectra of a C 60 3- molecule in a particle bath at finite temperature. The result is in qualitative agreement with the observed temperature dependence of the photoemission spectra of A 3 C 60 ." @default.
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• W1977176989 date "2002-02-15" @default.
• W1977176989 modified "2023-10-16" @default.
• W1977176989 title "Theoretical Study on Anomalous Behaviors in Photoemission Spectra of Alkali-Metal-Doped C60" @default.
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• W1977176989 doi "https://doi.org/10.1143/jpsj.71.525" @default.
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