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- W1977515468 abstract "The determination of phase transition temperatures for Cs-O mixtures containing up to 32 at% oxygen has established that the hitherto accepted phase diagram in the literature must be modified in the composition interval Cs7O-Cs7O2. Oxygen potentials in Cs-O liquids with 3.3 to 17 at% oxygen at 500–700°C have been determined by EMF measurements using ThO2−10 mol% Y2O3 electrolyte. The results were accurately described by the expression ΔḠO2 (J/mol O2) = −583800+ 156T+ 2RT (2140/T- 13) In x0 where R is the gas constant, T in K and 0 is the atomic fraction of oxygen. Caesium potentials at 500°C, derived from the above equation for x0 = 0−0.17 using the Duhem—Margules equation, were in excellent agreement with an extrapolation of caesium vapour pressure measurements by Arnol'dov et al. (x0 = 0.05–0.18, 280–360°C). Extrapolation of the oxygen potentials and derivation of the caesium potentials in the range 17–33.3 at% oxygen, combined with the results of Berardinelli and Kraus for higher oxygen concentrations provides an almost complete potential description of the Cs—O system up to 66 at% oxygen." @default.
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- W1977515468 date "1979-10-01" @default.
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- W1977515468 title "The Cs-O system;Phase diagram and oxygen potentials" @default.
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- W1977515468 doi "https://doi.org/10.1016/0022-3115(79)90163-6" @default.
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