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• W1977639781 abstract "A new, self-consistent formulation of the homogeneous nucleation theory has been proposed. This approach differs from the classical Becker-Döring-Zel'dovich theory in two respects: i) evaporation rates are evaluated by referring to the stable equilibrium of a saturated vapour rather than to the constrained metastable equilibrium of a supersaturated vapour; ii) for the reference stable equilibrium state the Fisher theory of condensation is used in order to obtain a self-consistent definition of the energy barrier for l-cluster formation. The present theory has no adjustable parameters. A comparison of the new expressions for the nucleation rate and critical cluster size with the corresponding classical expressions has been made for the different parts of the phase diagram (temperature-supersaturation) and the domain where both theories are close has been found. It has been shown that the present theory has much better agreement with experimental results for n-nonane than the classical one." @default.
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• W1977639781 date "1993-02-20" @default.
• W1977639781 modified "2023-09-27" @default.
• W1977639781 title "Cluster Approach to the Kinetic Theory of Homogeneous Nucleation" @default.
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• W1977639781 doi "https://doi.org/10.1209/0295-5075/21/6/002" @default.
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