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- W1977650240 startingPage "2020" @default.
- W1977650240 abstract "Direct numerical simulations are used to investigate the “long time” distribution of mass fraction fluctuations in stationary compressible isotropic turbulent binary nitrogen–hydrocarbon mixtures under supercritical pressure conditions. The governing equations are the compressible Navier–Stokes equations together with the cubic Peng–Robinson real gas state equation, and generalized heat and mass diffusion derived from nonequilibrium thermodynamics. A highly efficient procedure is presented which allows for the solution of all thermodynamic quantities without iterations or interpolation tables. The simulations consider equal mass binary mixtures of various combinations of nitrogen, heptane, dodecane, and 3-methylhexane, having molecular weight ratios in the range 1⩽MB/MA⩽6.08. It is shown that temperature and pressure-gradient-induced Soret mass diffusion results in statistically stationary mass fraction distributions at long times. The results reveal that the mass diffusion term due to the pressure gradient acts as a production mechanism in the Favre averaged scalar variance transport equation, and is balanced by Fickian dissipation to produce the stationary states. The resulting scalar probability density function is characterized by a larger than Gaussian flatness factor, and is asymmetric due to the mass fraction dependence of the partial molar volume. The stationary scalar variance amplitude increases both with increasing turbulence Mach number and molecular weight ratio of the species, but is inversely related to the turbulence Reynolds number. The scalar energy spectra exhibit peak values at wave numbers corresponding to the peak in the velocity dissipation spectra." @default.
- W1977650240 created "2016-06-24" @default.
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- W1977650240 date "2000-08-01" @default.
- W1977650240 modified "2023-09-24" @default.
- W1977650240 title "Long time mass fraction statistics in stationary compressible isotropic turbulence at supercritical pressure" @default.
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- W1977650240 doi "https://doi.org/10.1063/1.870448" @default.
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