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• W1977807162 abstract "The behavior of a linear polymer chain is studied in a solvent with high affinity for the polymer. The coil dimensions and specific heat are calculated as a function of chain length, solvent concentration, and polymer-solvent attraction strength εps. All other interactions are limited to excluded volume repulsion, which implies that the Flory–Huggins χ parameter is negative. Using both on-lattice and off-lattice models of a polymer chain in explicit solvent, we study a transition from weak to strong association regimes. In all cases studied, the system’s heat capacity is a nonmonotonic function of ερs with a maximum at attraction strengths of the order of several kBT. This peak originates from restriction of local conformational degrees of freedom due to the associated solvent rather than from a partial chain collapse which onsets as attractive solvent content is decreased." @default.
• W1977807162 created "2016-06-24" @default.
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• W1977807162 date "2008-11-05" @default.
• W1977807162 modified "2023-10-16" @default.
• W1977807162 title "Computer simulation study of a single polymer chain in an attractive solvent" @default.
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• W1977807162 doi "https://doi.org/10.1063/1.2991178" @default.
• W1977807162 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/19045372" @default.
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