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- W1977857535 endingPage "5083" @default.
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- W1977857535 abstract "We used dynamic light scattering (DLS) and computer simulations based on the fluctuating lattice Boltzmann equation (LBE) method to study the short-time Brownian dynamics of colloidal particles that interact like hard spheres. The dynamics are characterized by a Q-vector-dependent diffusion coefficient ${mathit{D}}_{mathit{S}}$(Q). Using DLS, we have mesaured ${mathit{D}}_{mathit{S}}$(Q) in the vicinity of the main (first) peak in the structure factor S(Q) for samples of poly-methylmethacrylate particles at volume fractions ensuremath{varphi} ranging from dilute up to the disorder-order transition (i.e., crystallization at ensuremath{varphi}=0.494). In addition we have determined the short-time self-diffusion (${mathit{D}}_{mathit{S}}^{mathit{S}}$) and collective-diffusion ${mathit{D}}_{mathit{S}}^{mathit{C}}$ coefficients. We have extracted the same quantities from simulations of equilibrium configurations of hard spheres using a fluctuating lattice Boltzmann equation method for the fluid phase coupled to Newtonian mechanics for the colloidal particles. For all samples studied, close quantitative agreement is found between the results of the DLS experiments and the LBE simulations." @default.
- W1977857535 created "2016-06-24" @default.
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- W1977857535 date "1995-11-01" @default.
- W1977857535 modified "2023-10-10" @default.
- W1977857535 title "Short-time Brownian motion in colloidal suspensions: Experiment and simulation" @default.
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- W1977857535 doi "https://doi.org/10.1103/physreve.52.5070" @default.
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