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- W1978133662 abstract "Diffuse reflectance FTIR spectroscopy was applied to the study of the fundamental C−O bond stretching vibrations and their first overtones and combination modes of copper carbonyl species formed upon CO adsorption on aqueous ion-exchanged CuZSM-5, CuM, CuY, and CuL zeolites autoreduced at 673 K in vacuo and on Cu(I)Y (sse) zeolite prepared by solid-state ion exchange of NH4Y with CuCl. At low CO pressures, different kinds of Cu(I)(CO) monocarbonyl species are formed depending upon the types of the zeolites. With increasing the CO pressure, Cu(I)(CO)2 dicarbonyl species are formed on CuZSM-5, CuM, and CuY. After an evacuation of the preadsorbed CO at room temperature, the dicarbonyl species are transformed into monocarbonyl species. Such a transformation is reversible upon a change of the CO pressure. On the CuL zeolite, however, only one type of monocarbonyl is observed, no dicarbonyl species being detected even at high CO pressures. The frequency of the stretching vibration of the metal cation−carbon bon..." @default.
- W1978133662 created "2016-06-24" @default.
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- W1978133662 date "1999-05-22" @default.
- W1978133662 modified "2023-10-17" @default.
- W1978133662 title "Investigation of Copper Carbonyl Species Formed upon CO Adsorption on Copper-Exchanged Zeolites by Diffuse Reflectance FTIR" @default.
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- W1978133662 doi "https://doi.org/10.1021/jp984727+" @default.
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