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• W1978207209 abstract "Methylated quartz surfaces are extensively used in colloid science for wettability studies and the control and impact of hydrophobicity in key physicochemical processes. In this study, time-of-flight secondary ion mass spectrometry (ToF-SIMS) has been used to correlate the surface chemistry of trimethylchlorosilane-methylated quartz surfaces with the contact angle. Models have been developed for the calculation of both advancing and receding contact angles based on measurements of the ToF-SIMS signals for SiC(3)H(9)(+) (TMCS) and Si(+) (quartz). These models enable the contact angle across surfaces and, more importantly, that of individual particles to be determined on a micrometer scale. Distributions of contact angles in large ensembles of particles, therefore, can now be determined. In addition, from the ToF-SIMS analysis, the surface coverage of the methylated species can be quantitatively determined, in line with the Cassie equation. Moreover, advancing and receding contact angle maps can be calculated from ToF-SIMS images, and hence the variation in microscopic hydrophobicity (e.g., at the particle level) can be extracted directly from the images." @default.
• W1978207209 created "2016-06-24" @default.
• W1978207209 creator A5014060065 @default.
• W1978207209 creator A5032922444 @default.
• W1978207209 date "2012-05-03" @default.
• W1978207209 modified "2023-10-14" @default.
• W1978207209 title "Determination of Contact Angles, Silane Coverage, and Hydrophobicity Heterogeneity of Methylated Quartz Surfaces Using ToF-SIMS" @default.
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• W1978207209 doi "https://doi.org/10.1021/la300352f" @default.
• W1978207209 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/22533310" @default.
• W1978207209 hasPublicationYear "2012" @default.
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