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- W1978277157 abstract "The optical absorption profile of an atom-surface vibrational bond is studied. From Markovian relaxation theory it follows that the line shape is a Lorentzian around the adsorbate resonance frequency ${mathrm{ensuremath{omega}}}_{0}$. Dispersion relations for crystals have a fairly small cutoff frequency ${mathrm{ensuremath{omega}}}_{mathrm{D}}$, which prohibits the use of such a simple theory. We calculated the spectral profile with finite--memory-time reservoir theory, and we found that the modified Lorentzian vanishes above ${mathrm{ensuremath{omega}}}_{mathrm{D}}$. Also a new spectral line at ${mathrm{ensuremath{omega}}}_{0}$+${mathrm{ensuremath{omega}}}_{mathrm{D}}$ is predicted, which disappears in the Markovian limit. The physical origin of the new line is explained." @default.
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- W1978277157 date "1988-04-11" @default.
- W1978277157 modified "2023-09-23" @default.
- W1978277157 title "Memory-induced extra resonances of adsorbates" @default.
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- W1978277157 doi "https://doi.org/10.1103/physrevlett.60.1487" @default.
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