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- W1978379218 abstract "We compare detailed dynamics of the excited-state absorption for C60 in solution, thin films, and entrapped in an inorganic sol-gel glass matrix. Our results demonstrate that the microscopic morphology of the C60 molecule plays a crucial role in determining the relaxation dynamics. This is a key factor for applications in optical limiting for nanosecond pulses using reverse saturable absorption. We find that the dynamics of the C60-glass composite occur on long timescales, comparable to that in solution; thin film samples, by contrast, show rapid decay. These results demonstrate that the C60-sol-gel glass composites contain C60 in a molecular dispersion, and are suitable candidates for solid-state optical limiting. Multispectral analysis of the decay dynamics in solution allows accurate determination of both the intersystem crossing time and the relative strengths of the singlet and triplet excited-state cross sections as a function of wavelength from 450-950 nm. The triplet excited-state cross section is greater than that for the singlet excited-state over the range form 620-810 nm." @default.
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- W1978379218 date "1996-12-16" @default.
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- W1978379218 title "<title>Femtosecond excited-state absorption dynamics and optical limiting in fullerene solutions, sol-gel glasses, and thin films</title>" @default.
- W1978379218 doi "https://doi.org/10.1117/12.262976" @default.
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