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• W1978406230 endingPage "1310" @default.
• W1978406230 startingPage "1301" @default.
• W1978406230 abstract "The HeI photoelectron spectra of the 12-vertex closo-1-SB11H11, 11-vertex nido-7-SB10H12 and nido-7,8,10-C2SB8H10, 10-vertex arachno-6,9-CSB8H12 and nine-vertex arachno-4-CB8H14 and arachno-4,6-C2B7H13 species are reported. The highest symmetry 1-thia closo species has the simplest spectrum: The five well-resolved band systems are assigned to F(surface), D(surface + BH), F(surface), P(BH) and F(BH) orbitals in the limit of spherical symmetry. The decrease of the symmetry in the open-face systems manifests itself in a greater complexity of photoelectron spectra and in the decrease of the first ionization energy by approximately 1 eV, due to the appearance of a new well-resolved band, The HOMO has a cluster surface bonding character in the open face systems. Going from closo to arachno clusters the contribution of hydrogen s functions in HOMO increases. For the arachno species a large H 1s contribution is found in low energy valence orbitals." @default.
• W1978406230 created "2016-06-24" @default.
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• W1978406230 date "1993-06-01" @default.
• W1978406230 modified "2023-10-18" @default.
• W1978406230 title "Electronic structure of heteroboranes derived from the icosahedral skeleton. UV photoelectron and MNDO study" @default.
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• W1978406230 doi "https://doi.org/10.1016/s0277-5387(00)84320-x" @default.
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