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• W1978482880 abstract "Boron is diamagnetic in B-doped anatase TiO2 nanoparticles which exhibit photocatalytic activities in the visible light range. Using N as a paramagnetic probe for the formal oxidation state of boron in N/B-codoped TiO2, with more than 90% unpaired spin density in the N2p orbital, we infer that boron enters the oxygen vacancy substitutionally in the form of B1-. Combination of spin-Hamiltonian analysis and interpretation of light dependent EPR spectra in terms of a charge compensating mechanism supports a model of [N2-B1-]+1 for the new EPR active center which acts as a trap for electrons liberated from [N1-] centers under blue light irradiation. Definite assignment of the boron oxidation state will contribute to the preparation, characterization, and understanding of B−TiO2 photoactivity under visible light which has been the subject of extensive work in the past few years." @default.
• W1978482880 created "2016-06-24" @default.
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• W1978482880 date "2008-02-07" @default.
• W1978482880 modified "2023-10-16" @default.
• W1978482880 title "Chemical State and Environment of Boron Dopant in B,N-Codoped Anatase TiO₂ Nanoparticles: An Avenue for Probing Diamagnetic Dopants in TiO₂ by Electron Paramagnetic Resonance Spectroscopy" @default.
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• W1978482880 doi "https://doi.org/10.1021/ja711424d" @default.
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