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- W1978514986 abstract "This study presents a three-dimensional numerical model that simulates the H 2 production from coal-derived syngas via a water-gas shift reaction in membrane reactors. The reactor was operated at a temperature of 900 °C, the typical syngas temperature at gasifier exit. The effects of membrane permeance, syngas composition, reactant residence time, sweep gas flow rate and steam-to-carbon (S/C) ratio on reactor performance were examined. Using CO conversion and H 2 recovery to characterize the reactor performance, it was found that the reactor performance can be enhanced using higher sweep gas flow rate, membrane permeance and S/C ratio. However, CO conversion and H 2 recovery limiting values were found when these parameters were further increased. The numerical results also indicated that the reactor performance degraded with increasing CO 2 content in the syngas composition. • 3-D numerical modeling on H 2 production via water-gas shift reaction in membrane reactor. • Limiting CO conversion and H 2 recovery resulted as the membrane permeance gets higher. • Limiting CO conversion and H 2 recovery can be found as the sweep gas flow rate increases. • Reactor performance degraded with increased CO 2 content in syngas. • For N 2 -contained syngas, reactor performance is controlled by the CO 2 content." @default.
- W1978514986 created "2016-06-24" @default.
- W1978514986 creator A5008478151 @default.
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- W1978514986 date "2014-09-01" @default.
- W1978514986 modified "2023-10-16" @default.
- W1978514986 title "Three-dimensional numerical modeling on high pressure membrane reactors for high temperature water-gas shift reaction" @default.
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- W1978514986 doi "https://doi.org/10.1016/j.ijhydene.2014.07.113" @default.
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