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• W1978521552 abstract "The reactions of [Ag(OH)4]− with aniline and xylidines have been investigated. The stopped-flow experiments reveal kinetically distinguishable steps involving initial complexation of the substrate with the silver(III) species which is followed by its decomposition. The latter process obeys first-order kinetics and takes place with a rate constant of about 0.8 s−1 through intramolecular electron transfer from substrate to the silver(III) center. Azobenzene and p-benzoquinone have been identified as the main products of the reaction of [Ag(OH)4]− and aniline. An increase in concentration of aniline enhances the yield of azobenzene which accounts for approximately 65% of the consumed aniline. This effect has been interpreted by the increased effective complexation between aniline and [Ag(OH)4]− at higher concentrations. The stoichiometry of the reaction is found to vary with a change in the concentration of aniline. At higher concentrations it comes out to be 1 : 2 for [Ag(OH)4]− : aniline. A mechanism of this reaction is worked out." @default.
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• W1978521552 date "1994-05-01" @default.
• W1978521552 modified "2023-09-25" @default.
• W1978521552 title "Kinetics of Oxidation of Aniline and Xylidines by the Tetrahydroxoargentate(III) Ion" @default.
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• W1978521552 doi "https://doi.org/10.1246/bcsj.67.1207" @default.
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